Preparation of a Novel Chitosan Based Biopolymer Dye and Application in Wood Dyeing.
Identifieur interne : 001704 ( Main/Exploration ); précédent : 001703; suivant : 001705Preparation of a Novel Chitosan Based Biopolymer Dye and Application in Wood Dyeing.
Auteurs : Xiaoqian Wang [République populaire de Chine] ; Ruilin Tang [République populaire de Chine] ; Yang Zhang [République populaire de Chine] ; Zhiming Yu [République populaire de Chine] ; Chusheng Qi [République populaire de Chine]Source :
- Polymers [ 2073-4360 ] ; 2016.
Abstract
A novel chitosan-based biopolymer dye possessing antibacterial properties was synthesized by reaction of O-carboxymethyl chitosan and Acid Red GR. The synthesized materials were characterized by Fourier transform infrared spectroscopy (FTIR), degree of substitution (DS), X-ray photoelectron spectroscopy (XPS), thermogravimetric analysis (TG), X-ray diffraction (XRD), water solubility test, antibacterial property test, and dyeing performance, including dye uptake, color difference, and fastness. Results showed that the synthesized dye was combined by ⁻NH₃⁺ of O-carboxymethyl chitosan and the sulfonic group of Acid Red GR. According to the comprehensive analysis of XRD and water solubility, the introduction of the carboxymethyl group and acid dye molecule changed the structure of the chitosan from compact to loose, which improved the synthesized dye's water solubility. However, the thermal stability of the synthesized dye was decreased. The antibacterial property of the poplar wood dyed with the synthesized dye was enhanced and its antibacterial rate, specifically against Staphylococcus aureus and Escherichia coli, also increased to a rate of more than 99%. However, the dye uptake of the synthesized dye was lower than that of the original dye. Despite this, though, the dyeing effect of the synthesized dye demonstrated better water-fastness, and light-fastness than the original dye. Therefore, the novel chitosan-based biopolymer dye can be a promising product for wood dyeing.
DOI: 10.3390/polym8090338
PubMed: 30974613
PubMed Central: PMC6431893
Affiliations:
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Chine</country><wicri:regionArea>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083</wicri:regionArea><placeName><settlement type="city">Pékin</settlement></placeName></affiliation><affiliation wicri:level="1"><nlm:affiliation>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083, China. xiaoqianwang1@126.com.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083</wicri:regionArea><placeName><settlement type="city">Pékin</settlement></placeName></affiliation></author><author><name sortKey="Tang, Ruilin" sort="Tang, Ruilin" uniqKey="Tang R" first="Ruilin" last="Tang">Ruilin Tang</name><affiliation wicri:level="1"><nlm:affiliation>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China. tangruilin@bjfu.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083</wicri:regionArea><placeName><settlement type="city">Pékin</settlement></placeName></affiliation><affiliation wicri:level="1"><nlm:affiliation>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083, China. tangruilin@bjfu.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083</wicri:regionArea><placeName><settlement type="city">Pékin</settlement></placeName></affiliation></author><author><name sortKey="Zhang, Yang" sort="Zhang, Yang" uniqKey="Zhang Y" first="Yang" last="Zhang">Yang Zhang</name><affiliation wicri:level="1"><nlm:affiliation>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China. bjfuzhangyang@bjfu.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083</wicri:regionArea><placeName><settlement type="city">Pékin</settlement></placeName></affiliation><affiliation wicri:level="1"><nlm:affiliation>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083, China. bjfuzhangyang@bjfu.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083</wicri:regionArea><placeName><settlement type="city">Pékin</settlement></placeName></affiliation></author><author><name sortKey="Yu, Zhiming" sort="Yu, Zhiming" uniqKey="Yu Z" first="Zhiming" last="Yu">Zhiming Yu</name><affiliation wicri:level="1"><nlm:affiliation>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China. yuzhiming@bjfu.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083</wicri:regionArea><placeName><settlement type="city">Pékin</settlement></placeName></affiliation><affiliation wicri:level="1"><nlm:affiliation>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083, China. yuzhiming@bjfu.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083</wicri:regionArea><placeName><settlement type="city">Pékin</settlement></placeName></affiliation></author><author><name sortKey="Qi, Chusheng" sort="Qi, Chusheng" uniqKey="Qi C" first="Chusheng" last="Qi">Chusheng Qi</name><affiliation wicri:level="1"><nlm:affiliation>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China. qichusheng@bjfu.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083</wicri:regionArea><placeName><settlement type="city">Pékin</settlement></placeName></affiliation><affiliation wicri:level="1"><nlm:affiliation>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083, China. qichusheng@bjfu.edu.cn.</nlm:affiliation><country xml:lang="fr">République populaire de Chine</country><wicri:regionArea>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083</wicri:regionArea><placeName><settlement type="city">Pékin</settlement></placeName></affiliation></author></analytic><series><title level="j">Polymers</title><idno type="eISSN">2073-4360</idno><imprint><date when="2016" type="published">2016</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">A novel chitosan-based biopolymer dye possessing antibacterial properties was synthesized by reaction of <i>O</i>-carboxymethyl chitosan and Acid Red GR. The synthesized materials were characterized by Fourier transform infrared spectroscopy (FTIR), degree of substitution (DS), X-ray photoelectron spectroscopy (XPS), thermogravimetric analysis (TG), X-ray diffraction (XRD), water solubility test, antibacterial property test, and dyeing performance, including dye uptake, color difference, and fastness. Results showed that the synthesized dye was combined by ⁻NH₃⁺ of <i>O</i>-carboxymethyl chitosan and the sulfonic group of Acid Red GR. According to the comprehensive analysis of XRD and water solubility, the introduction of the carboxymethyl group and acid dye molecule changed the structure of the chitosan from compact to loose, which improved the synthesized dye's water solubility. However, the thermal stability of the synthesized dye was decreased. The antibacterial property of the poplar wood dyed with the synthesized dye was enhanced and its antibacterial rate, specifically against <i>Staphylococcus aureus</i> and <i>Escherichia coli</i>, also increased to a rate of more than 99%. However, the dye uptake of the synthesized dye was lower than that of the original dye. Despite this, though, the dyeing effect of the synthesized dye demonstrated better water-fastness, and light-fastness than the original dye. Therefore, the novel chitosan-based biopolymer dye can be a promising product for wood dyeing.</div></front></TEI><pubmed><MedlineCitation Status="PubMed-not-MEDLINE" Owner="NLM"><PMID Version="1">30974613</PMID><DateRevised><Year>2020</Year><Month>09</Month><Day>30</Day></DateRevised><Article PubModel="Electronic"><Journal><ISSN IssnType="Electronic">2073-4360</ISSN><JournalIssue CitedMedium="Internet"><Volume>8</Volume><Issue>9</Issue><PubDate><Year>2016</Year><Month>Sep</Month><Day>10</Day></PubDate></JournalIssue><Title>Polymers</Title><ISOAbbreviation>Polymers (Basel)</ISOAbbreviation></Journal><ArticleTitle>Preparation of a Novel Chitosan Based Biopolymer Dye and Application in Wood Dyeing.</ArticleTitle><ELocationID EIdType="pii" ValidYN="Y">E338</ELocationID><ELocationID EIdType="doi" ValidYN="Y">10.3390/polym8090338</ELocationID><Abstract><AbstractText>A novel chitosan-based biopolymer dye possessing antibacterial properties was synthesized by reaction of <i>O</i>-carboxymethyl chitosan and Acid Red GR. The synthesized materials were characterized by Fourier transform infrared spectroscopy (FTIR), degree of substitution (DS), X-ray photoelectron spectroscopy (XPS), thermogravimetric analysis (TG), X-ray diffraction (XRD), water solubility test, antibacterial property test, and dyeing performance, including dye uptake, color difference, and fastness. Results showed that the synthesized dye was combined by ⁻NH₃⁺ of <i>O</i>-carboxymethyl chitosan and the sulfonic group of Acid Red GR. According to the comprehensive analysis of XRD and water solubility, the introduction of the carboxymethyl group and acid dye molecule changed the structure of the chitosan from compact to loose, which improved the synthesized dye's water solubility. However, the thermal stability of the synthesized dye was decreased. The antibacterial property of the poplar wood dyed with the synthesized dye was enhanced and its antibacterial rate, specifically against <i>Staphylococcus aureus</i> and <i>Escherichia coli</i>, also increased to a rate of more than 99%. However, the dye uptake of the synthesized dye was lower than that of the original dye. Despite this, though, the dyeing effect of the synthesized dye demonstrated better water-fastness, and light-fastness than the original dye. Therefore, the novel chitosan-based biopolymer dye can be a promising product for wood dyeing.</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Wang</LastName><ForeName>Xiaoqian</ForeName><Initials>X</Initials><Identifier Source="ORCID">0000-0001-6212-1789</Identifier><AffiliationInfo><Affiliation>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China. xiaoqianwang1@126.com.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083, China. xiaoqianwang1@126.com.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Tang</LastName><ForeName>Ruilin</ForeName><Initials>R</Initials><AffiliationInfo><Affiliation>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China. tangruilin@bjfu.edu.cn.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083, China. tangruilin@bjfu.edu.cn.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zhang</LastName><ForeName>Yang</ForeName><Initials>Y</Initials><AffiliationInfo><Affiliation>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China. bjfuzhangyang@bjfu.edu.cn.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083, China. bjfuzhangyang@bjfu.edu.cn.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Yu</LastName><ForeName>Zhiming</ForeName><Initials>Z</Initials><AffiliationInfo><Affiliation>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China. yuzhiming@bjfu.edu.cn.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083, China. yuzhiming@bjfu.edu.cn.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Qi</LastName><ForeName>Chusheng</ForeName><Initials>C</Initials><AffiliationInfo><Affiliation>Beijing Key Laboratory of Wood Science and Engineering, Beijing Forestry University, Beijing 100083, China. qichusheng@bjfu.edu.cn.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Ministry of Education Key Laboratory of Wooden Material Science and Application, Beijing Forestry University, Beijing 100083, China. qichusheng@bjfu.edu.cn.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><GrantList CompleteYN="Y"><Grant><Agency>Co-built Project Beijing Municipal Education Commission (2016) "R ＆ D on Technology in Scientific Utilization of Non-wood Plant Material"</Agency><Country></Country></Grant><Grant><GrantID>No. 2016ZCQ01, BLYJ201626 and 2016BLRD03</GrantID><Agency>Fundamental Research Funds for the Central Universities</Agency><Country></Country></Grant></GrantList><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2016</Year><Month>09</Month><Day>10</Day></ArticleDate></Article><MedlineJournalInfo><Country>Switzerland</Country><MedlineTA>Polymers (Basel)</MedlineTA><NlmUniqueID>101545357</NlmUniqueID><ISSNLinking>2073-4360</ISSNLinking></MedlineJournalInfo><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">O-carboxymethyl chitosan</Keyword><Keyword MajorTopicYN="N">antibacterial activity</Keyword><Keyword MajorTopicYN="N">dye</Keyword><Keyword MajorTopicYN="N">dyeing performance</Keyword><Keyword MajorTopicYN="N">preparation</Keyword><Keyword MajorTopicYN="N">water solubility</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2016</Year><Month>06</Month><Day>30</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2016</Year><Month>08</Month><Day>22</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2016</Year><Month>09</Month><Day>07</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2019</Year><Month>4</Month><Day>13</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2016</Year><Month>9</Month><Day>10</Day><Hour>0</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="medline"><Year>2016</Year><Month>9</Month><Day>10</Day><Hour>0</Hour><Minute>1</Minute></PubMedPubDate></History><PublicationStatus>epublish</PublicationStatus><ArticleIdList><ArticleId IdType="pubmed">30974613</ArticleId><ArticleId IdType="pii">polym8090338</ArticleId><ArticleId IdType="doi">10.3390/polym8090338</ArticleId><ArticleId 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first="Xiaoqian" last="Wang">Xiaoqian Wang</name></noRegion><name sortKey="Qi, Chusheng" sort="Qi, Chusheng" uniqKey="Qi C" first="Chusheng" last="Qi">Chusheng Qi</name><name sortKey="Qi, Chusheng" sort="Qi, Chusheng" uniqKey="Qi C" first="Chusheng" last="Qi">Chusheng Qi</name><name sortKey="Tang, Ruilin" sort="Tang, Ruilin" uniqKey="Tang R" first="Ruilin" last="Tang">Ruilin Tang</name><name sortKey="Tang, Ruilin" sort="Tang, Ruilin" uniqKey="Tang R" first="Ruilin" last="Tang">Ruilin Tang</name><name sortKey="Wang, Xiaoqian" sort="Wang, Xiaoqian" uniqKey="Wang X" first="Xiaoqian" last="Wang">Xiaoqian Wang</name><name sortKey="Yu, Zhiming" sort="Yu, Zhiming" uniqKey="Yu Z" first="Zhiming" last="Yu">Zhiming Yu</name><name sortKey="Yu, Zhiming" sort="Yu, Zhiming" uniqKey="Yu Z" first="Zhiming" last="Yu">Zhiming Yu</name><name sortKey="Zhang, Yang" sort="Zhang, Yang" uniqKey="Zhang Y" first="Yang" last="Zhang">Yang Zhang</name><name sortKey="Zhang, Yang" sort="Zhang, Yang" uniqKey="Zhang Y" first="Yang" last="Zhang">Yang Zhang</name></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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